Assuming that you're running at an easy pace and drinking water during your long run, what you're describing at the 110-120 minute point is the classic symptom of glycogen exhaustion: running out of glycogen. You're hitting, or gliding into, the wall.
And that's just fine. It's good, in fact. Now you know exactly where your current limit is.
At that moment, when your glycogen runs out, your body is trying to switch over to 100% fat burning. It is not a comfortable feeling! But the more you prepare yourself for the switchover, psychologically, the easier it will be to accept what has happened. Just slow down, adjust your breathing, allow your heart rate to stabilize, and keep on going. Run at least 10-15 minutes past that point. In my experience, your body slowly begins to learn how to accommodate itself to the demand. And if you continue to alternate long runs of 1:55-2:05 with longer long runs of 2:30 or so, the boundary will slowly slide back. You'll hit two hours and won't hit the wall.
Do make sure that you're hydrating properly. I do ALL my long runs, up to three hours, with NO carbs either before or during the run, so I know it's possible. McMillan teaches that long slow runs of up to three hours help get your body used to fat burning.
Only by going beyond the point of glycogen exhaustion and VALUING the experience, dragged-out as you may feel, will you slowly train your body to pack on the glycogen.
You can absolutely to this. Learn to appreciate and actually value the moment when your body is switching from part-glycogen to 100% fat burning. The bad/sick/exhausted feelings will pass. Your body will stabilize. But you need to go easy, especially when you're first pushing out your boundaries.